"Evidence For Luttinger Liquid Physics in Dimension Higher Than One from ARPES of Li0.9Mo6O17"

 

J.W. Allen
University of Michigan

Li0.9Mo6O17is a quasi-one dimensional (1D) superconducting metal whose single particle spectrum as measured by angle resolved photoemission spectroscopy (ARPES) has features generic to the T-dependent spectral function of the one-band Tomonaga-Luttinger model.  The ARPES spectrum of the dispersing excitation defining its quasi-1D Fermi surface shows a holon (charge mode) peak and a spinon edge dispersing with different velocities, and the k-integrated spectrum approaches the Fermi energy EF as a power law with anomalous exponent a.  A strong T-dependence of a [1] and the particulars of quantum critical scaling observed in the ARPES spectrum [2] can be traced to interacting gapped charge neutral critical modes that emerge naturally for Li0.9Mo6O17 because two nearly degenerate bands cross EF. New band structure calculations and additional ARPES results conspire to imply the presence of a mechanism for suppression of perpendicular hopping that would otherwise destabilize the observed Luttinger liquid (LL) behavior.  Such a mechanism would constitute a scenario for a new quantum state of matter in which LL physics is maintained in dimension greater than one.

[1] Feng Wang et al., “New Luttinger-Liquid Physics from Photoemission on Li0.9Mo6O17,” Phys. Rev. Lett. 96, 196403 (2006).
[2]  J. V. Alvarez et al, "Gap-protected Quantum Critical Scaling in ARPES of Li0.9Mo6O17," submitted to Phys. Rev. Lett.

* Collaborators: J. V. Alvarez (Univ. Autonoma Madrid),  Feng Wang (Univ. of Michigan), S.-K. Mo (Stanford Univ.), G.-H. Gweon (Univ. of California, Santa Cruz), J. He (Clemson Univ.) , D. Mandrus (Univ. of Tennessee and Oak Ridge National Lab), R. Jin (ORNL), and H. Höchst (SRC, Univ. of Wisconsin).


Updated: Tue, 01-Apr-2008 11:50 AM